Somatic mutations in ACVR1, encoding the serine/threonine kinase ALK2, are prevalent in 20-25% of DMG-H3K27M patients. While ALK2 inhibitors (ALK2i) extend survival in ACVR1-mutant orthotopic xenografts, these inhibitors do not achieve complete tumour regression as monotherapy. To uncover novel combination strategies, an international collaborative effort combined resources to evaluate the novel ALK2i TP-0184 across a large panel of patient-derived DMG-H3K27 models in vitro, revealing IC50 values ranging from approximately 0.5 to 10 mM, irrespective of ACVR1 mutation status. Western blot analysis demonstrated the inhibition of phospho-SMAD1/5/9 and PI3K following TP-0184 treatment. Synergistic interactions were observed between TP-0184 and the MEK inhibitor trametinib in ACVR1-mutant DMG models in flow cytometric analysis for apoptosis and in vitro cytotoxicity assays. Importantly, combining TP-0184 with radiation in vitro demonstrated profound radiosensitisation effects in three ACVR1-mutant models, as corroborated by clonogenic assays and increased gH2AX levels and cleaved caspase 3 using western blotting. Animal studies determined the tolerable dosing regimen for TP-0184, either alone or in combination with trametinib, with the optimal doses established at 100 mg/kg/day for TP-0184 and 0.4 mg/kg/day for trametinib. In vivo efficacy studies using an orthotopic DMG model harbouring ACVR1 mutation revealed a moderate yet significantly enhanced median survival (61 days) with TP0184 monotherapy compared to vehicle control (56 days). Notably, combining TP-0184 with either irradiation or trametinib further extended animal survival (71 days for TP-0184/Trametinib and 79 days for TP0184/Irradiation) compared to single-agent treatments (67 days for irradiation and 59.5 days for trametinib). Ongoing in vivo studies involving additional DMG-H3K27 models across multiple laboratories are underway to assess the combination of TP-0184 with trametinib and radiation comprehensively. These findings have led to the inclusion of both TP-0184 combinatorial approaches as treatment arms in the TARGET precision-guided clinical trial for paediatric high-grade gliomas, coordinated internationally through the CONNECT consortium.